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- W4315436771 abstract "Metal-oxide interaction was widely observed in supported metal catalysts, playing a significant role in tuning the catalytic performance. Here, we reported that the interaction of Ru and MnOx was able to facilitate the hydrodeoxygenation of levulinic acid (LA) to 2-butanol with a high turnover frequency (1.99 × 106 h-1), turnover number (4411), and yield (98.8%). Moreover, this catalyst was capable of removing the hydroxymethyl group of lactones and diol with high yields of products. The high activity of the Ru-MnOx catalyst was due to the strong Ru-MnOx interaction, which facilitated reduction of Ru oxide to Ru0 and Mn oxide to Mn2+. The increased fractions of Ru0 and Mn2+ provided metal and Lewis acid sites, respectively, and therefore facilitated LA hydrodeoxygenation. A linear correlation between the hydrodeoxygenation activity of the Ru-MnOx catalyst and [Mn2+]ln([Ru0]) was observed." @default.
- W4315436771 created "2023-01-11" @default.
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- W4315436771 date "2023-01-10" @default.
- W4315436771 modified "2023-10-13" @default.
- W4315436771 title "Ru–MnO<sub><i>x</i></sub> Interaction for Efficient Hydrodeoxygenation of Levulinic Acid and Its Derivatives" @default.
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- W4315436771 doi "https://doi.org/10.1021/acsami.2c22045" @default.
- W4315436771 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36626197" @default.
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