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• W4315465017 abstract "Abstract It is highly desired to achieve controllable product selectivity in CO 2 hydrogenation. Herein, we report light‐induced switching of reaction pathways of CO 2 hydrogenation towards CH 3 OH production over actomically dispersed Co decorated Pt@UiO‐66‐NH 2 . CO, being the main product in the reverse water gas shift (RWGS) pathway under thermocatalysis condition, is switched to CH 3 OH via the formate pathway with the assistance of light irradiation. Impressively, the space‐time yield of CH 3 OH in photo‐assisted thermocatalysis (1916.3 μmol g cat −1 h −1 ) is about 7.8 times higher than that without light at 240 °C and 1.5 MPa. Mechanism investigation indicates that upon light irradiation, excited UiO‐66‐NH 2 can transfer electrons to Pt nanoparticles and Co sites, which can efficiently catalyze the critical elementary steps (i.e., CO 2 ‐to‐*HCOO conversion), thus suppressing the RWGS pathway to achieve a high CH 3 OH selectivity." @default.
• W4315465017 created "2023-01-11" @default.
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• W4315465017 date "2023-01-24" @default.
• W4315465017 modified "2023-09-26" @default.
• W4315465017 title "Photo‐Induced Switching of CO₂ Hydrogenation Pathway towards CH₃OH Production over Pt@UiO‐66‐NH₂(Co)" @default.
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• W4315465017 doi "https://doi.org/10.1002/ange.202218115" @default.
• W4315465017 hasPublicationYear "2023" @default.
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