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- W4315478091 abstract "Metal halides (MHs) show great potential in photovoltaic and optoelectronic applications, but their lack of long-term stability limits their applications for their sensitivity to oxygen, moisture, strong light irradiation, and high temperature. In this report, lead-free MHs CsCu2I3/Cs3Cu2I5 dual-phase glass-ceramics were prepared with a traditional melting-quenching method by using solid reductive agent Si3N4. Ultrabroadband emission from violet to near-infrared (350–800 nm) can be obtained from these CsCu2I3/Cs3Cu2I5 dual-phase glass-ceramics with long-term water-resistance stability. Detailed analysis of microstructure, spectra, and calculation reveals that the ultrabroadband nature can be ascribed to the intense emission of CsCu2I3 NCs, Cu+ ions, and Cs3Cu2I5 NCs together, and especially, the emission from Cs3Cu2I5 NCs and Cu+ ions presents a cyan color. Our work not only demonstrates that CsCu2I3/Cs3Cu2I5 glass-ceramic is a promising fluorescent material, but also develops a method to prepare lead-free metal halides CsCu2I3/Cs3Cu2I5 dual-phase glass-ceramics with high stability, paving the way for their applications." @default.
- W4315478091 created "2023-01-11" @default.
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- W4315478091 date "2023-01-10" @default.
- W4315478091 modified "2023-10-15" @default.
- W4315478091 title "Ultrabroadband Emission from CsCu<sub>2</sub>I<sub>3</sub>/Cs<sub>3</sub>Cu<sub>2</sub>I<sub>5</sub> Dual-Phase Glass-Ceramics with Long-Term Stability" @default.
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- W4315478091 doi "https://doi.org/10.1021/acsaom.2c00127" @default.
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