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- W4315703059 abstract "Acetic acid/acetate is an important precursor for many chemical manufacturing sectors, as well as a feedstock for the microbial synthesis of value-added biofuel and biomass products. As the downstream reaction in tandem with the carbon dioxide reduction reaction, carbon monoxide electrolysis has a unique advantage over direct carbon dioxide reduction, boosting the selectivity for multicarbon products. However, highly selective and high-current-throughput acetate and 1-propanol production from CO electrolysis is yet to be explored. Herein, we present practical approaches for improving acetate and 1-propanol selectivity and yield from CO electrolysis using a commercial copper catalyst. Acetate showed a strong pH dependence with an optimum performance at 90% Faradaic efficiency and 128 mA cm–2 current density. In addition, 1-propanol showed a strong catalyst loading dependence, achieving 20% Faradaic efficiency under high-catalyst-loading conditions. In situ Raman and Multiphysics modeling further demonstrated the mechanism of the improvements." @default.
- W4315703059 created "2023-01-12" @default.
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- W4315703059 date "2023-01-12" @default.
- W4315703059 modified "2023-10-13" @default.
- W4315703059 title "Promoting Electrolysis of Carbon Monoxide toward Acetate and 1-Propanol in Flow Electrolyzer" @default.
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- W4315703059 doi "https://doi.org/10.1021/acsenergylett.2c02502" @default.
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