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• W4316590803 abstract "Abstract The inner-valence ionization and fragmentation dynamics of CH 4 –C 6 H 6 dimer induced by 200 eV electron impact is studied utilizing a multi-particle coincidence momentum spectroscopy. The three-dimensional momentum vectors and kinetic energy release (KER) of the CH 4 + +C 6 H 6 + ion pairs are obtained by coincident momentum measurement. Our analysis on the absolute cross sections indicates that the intermediate dication CH 4 + –C 6 H 6 + is preferentially produced by the removal of an inner-valence electron from CH 4 or C 6 H 6 and subsequent relaxation of ultrafast intermolecular Coulombic decay followed by two-body Coulomb explosion. Combining with ab initio molecular dynamics (AIMD) simulations, the real-time fragmentation dynamics including translational, vibrational and rotational motions are presented as a function of propagation time. The revealed fragmentation dynamics are expected to have a potential implication for crystal structure imaging with various radiation sources." @default.
• W4316590803 created "2023-01-17" @default.
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• W4316590803 date "2023-02-09" @default.
• W4316590803 modified "2023-09-24" @default.
• W4316590803 title "Structural and dynamical studies of CH–π bonded CH₄–C₆H₆ dimer by ultrafast intermolecular Coulombic decay" @default.
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• W4316590803 doi "https://doi.org/10.1088/1361-6528/acb358" @default.
• W4316590803 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36645904" @default.
• W4316590803 hasPublicationYear "2023" @default.
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