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• W4316653295 abstract "Abstract Enhancing the peroxymonosulfate (PMS) activation efficiency to generate more radicals is vital to promote the Fenton‐like reaction activity, however, how to promote the PMS adsorption and accelerate the interfacial electron transfer to boost its activation kinetics remains a great challenge. Herein, we prepared Cu‐doped defect‐rich In 2 O 3 (Cu‐In 2 O 3 /O v ) catalysts containing asymmetric Cu−O v −In sites for PMS activation in water purification. The intrinsic catalytic activity is that the side‐on adsorption configuration of the O−O bond (Cu−O−O−In) at the Cu‐O v ‐In sites significantly stretches the O−O bond length. Meanwhile, the Cu‐O v ‐In sites increase the electron density near the Fermi energy level, promoting more and faster electron transfer to the O−O bond for generating more SO 4 ⋅ − and ⋅OH. The degradation rate constant of tetracycline achieved by Cu‐In 2 O 3 /O v is 31.8 times faster than In 2 O 3 /O v , and it shows the possibility of membrane reactor for practical wastewater treatment." @default.
• W4316653295 created "2023-01-17" @default.
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• W4316653295 date "2023-02-01" @default.
• W4316653295 modified "2023-10-17" @default.
• W4316653295 title "Enhanced Interfacial Electron Transfer by Asymmetric Cu‐O_v‐In Sites on In₂O₃ for Efficient Peroxymonosulfate Activation" @default.
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• W4316653295 doi "https://doi.org/10.1002/ange.202216403" @default.
• W4316653295 hasPublicationYear "2023" @default.
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