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• W4316925801 abstract "Conventional cathodes generally store charges inside solids, and they usually suffer from compromised performance at low temperatures due to the energy barriers for ion transport. Here we report a reversible “plating” reaction of Cl2 liquid inside nanoporous carbon as a new electrode for low-temperature aqueous batteries. In a 7 m LiCl aqueous electrolyte, the activated carbon electrode delivers a high discharge capacity of 475 mAh/g (based on the carbon active mass in the working electrode) at 100 mA/g at −78 °C with a discharging plateau at ca. 0.95 V vs Ag/AgCl and retains a high capacity of 238 mAh/g at a high current rate of 1 A/g. Furthermore, this electrode system demonstrates stable cycling with ca. 65% capacity retention after 100 cycles at 500 mA/g with an average Coulombic efficiency of above 99%. The results provide a new option for high-energy halogen cathodes at low temperatures." @default.
• W4316925801 created "2023-01-18" @default.
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• W4316925801 date "2023-01-17" @default.
• W4316925801 modified "2023-10-17" @default.
• W4316925801 title "Reversible Cl₂/Cl^– Redox for Low-Temperature Aqueous Batteries" @default.
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• W4316925801 doi "https://doi.org/10.1021/acsenergylett.2c02757" @default.
• W4316925801 hasPublicationYear "2023" @default.
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