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- W4317106072 abstract "New strategies for the design and synthesis of stable organic radicals without additives are highly desirable. Herein, we design a series of donor-acceptor structured triarylphosphines and disclose the fast color change triggered by UV-irradiation in the crystalline state. Photoinduced organic radicals are undoubtedly verified and proved to be the reason for the color change by time-dependent and quantitative electron paramagnetic resonance analysis, X-ray crystallographic analysis, and theoretical calculations. It is revealed that the intrinsic symmetry breaking of peripheral architecture helps to form continuous molecular chains by donor-acceptor counterpart pairing. Intermolecular electron-transfer occurs among molecular chains and results in radical ion pairs upon photoirradiation." @default.
- W4317106072 created "2023-01-18" @default.
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- W4317106072 date "2023-01-01" @default.
- W4317106072 modified "2023-10-01" @default.
- W4317106072 title "Manipulating D–A interaction to achieve stable photoinduced organic radicals in triphenylphosphine crystals" @default.
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- W4317106072 doi "https://doi.org/10.1039/d2sc05753k" @default.
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