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• W4317605841 endingPage "2209310" @default.
• W4317605841 startingPage "2209310" @default.
• W4317605841 abstract "Single-atom catalysts have become a popular choice in various catalysis applications, as they take advantages of both homogeneous catalysis (e.g., high efficiency) and heterogeneous catalysis (e.g., easy catalyst recovery). The atom support plays an indispensable role in anchoring atomic species and interplaying with them for ultimate catalytic performance. Therefore, development of new support materials for superior catalysis is of great importance. Here the synthesis of carbon nanofibers based on the reaction between phosphorus pentoxide (P2O5) and N-methyl-2-pyrrolidone (NMP) is reported. The underlying reaction process is systematically investigated by Fourier-transform infrared (FTIR) spectroscopy and nuclear magnetic resonance (NMR) spectroscopy. The carbon nanofibers have interesting PN units in their chemical structure, which act as anchoring sites for the single-atom catalyst. The Pt atoms anchoring carbon nanofibers exhibit high activity for hydrosilylation with a turnover frequency (TOF) of 9.2 × 106 h−1 and a selectivity of >99%. This research affords not only a new in situ chemical strategy to synthesize multiatom doped carbon nanofibers but also presents a potential superior support in catalysis, which opens a hopeful window in materials chemistry and catalysis applications." @default.
• W4317605841 created "2023-01-21" @default.
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• W4317605841 date "2023-03-04" @default.
• W4317605841 modified "2023-10-17" @default.
• W4317605841 title "In‐Situ Synthesis of PN‐Doped Carbon Nanofibers for Single‐Atom Catalytic Hydrosilylation" @default.
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• W4317605841 doi "https://doi.org/10.1002/adma.202209310" @default.
• W4317605841 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36670489" @default.
• W4317605841 hasPublicationYear "2023" @default.
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