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- W4317666419 endingPage "119064" @default.
- W4317666419 startingPage "119064" @default.
- W4317666419 abstract "The transformation of lignocellulosic biomass to platform compounds (γ-valerolactone, GVL) was a significant component in biomass development. Herein, sulfonated Zr-based metal-organic frameworks (MOF-808), a bifunctional heterogeneous catalyst with Lewis and Bronsted acid sites, were prepared to catalyze the one-pot cascade reaction of furfural (FUR) to GVL. The successful modification of the sulfonic group on MOF-808 was substantiated by multiple characterization methods. By adjusting the sulfuric acid concentration to balance the Lewis acid and Bronsted acid sites of the catalyst, S-808–2.37 was confirmed as the preferred catalyst and a 60.4 % GVL yield was achieved with 99.1 % carbon balance under the optimal conditions. Moreover, the 72.8 % GVL yield reached in the 40x magnification experiment also boded well for the catalyst’s application potential. The work in this paper opened up new perspectives for the application of MOF-808 porous materials in the field of selective catalytic conversion of biomass involving multi-step reactions." @default.
- W4317666419 created "2023-01-21" @default.
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- W4317666419 date "2023-03-01" @default.
- W4317666419 modified "2023-09-27" @default.
- W4317666419 title "Bifunctional zirconium-based metal-organic frameworks as chemoselective catalysts for the synthesis of γ-valerolactone from furfural via a one-pot cascade reaction" @default.
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- W4317666419 doi "https://doi.org/10.1016/j.apcata.2023.119064" @default.
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