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- W4317776973 abstract "Abstract The electrochemical nitrogen (N 2 ) reduction reaction (N 2 RR) under mild conditions is a promising and environmentally friendly alternative to the traditional Haber‐Bosch process with high energy consumption and greenhouse emission for the synthesis of ammonia (NH 3 ), but high‐yielding production is rendered challenging by the strong nonpolar N≡N bond in N 2 molecules, which hinders their dissociation or activation. In this study, disordered Au nanoclusters anchored on two‐dimensional ultrathin Ti 3 C 2 T x MXene nanosheets are explored as highly active and selective electrocatalysts for efficient N 2 ‐to‐NH 3 conversion, exhibiting exceptional activity with an NH 3 yield rate of 88.3±1.7 μg h −1 mg cat. −1 and a faradaic efficiency of 9.3±0.4 %. A combination of in situ near‐ambient pressure X‐ray photoelectron spectroscopy and operando X‐ray absorption fine structure spectroscopy is employed to unveil the uniqueness of this catalyst for N 2 RR. The disordered structure is found to serve as the active site for N 2 chemisorption and activation during the N 2 RR process." @default.
- W4317776973 created "2023-01-24" @default.
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- W4317776973 date "2023-02-08" @default.
- W4317776973 modified "2023-10-15" @default.
- W4317776973 title "Disordered Au Nanoclusters for Efficient Ammonia Electrosynthesis" @default.
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- W4317776973 doi "https://doi.org/10.1002/cssc.202201385" @default.
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