Matches in SemOpenAlex for { <https://semopenalex.org/work/W4317937914> ?p ?o ?g. }
- W4317937914 endingPage "232651" @default.
- W4317937914 startingPage "232651" @default.
- W4317937914 abstract "The solid-electrolyte interphase (SEI) substantially influences the lifetime of lithium-ion batteries. Nevertheless, the transport mechanism responsible for the long-term growth of the SEI remains controversial. This study aims at discussing the characteristic time and state-of-charge dependence of SEI growth mediated by electron diffusion versus solvent diffusion. We describe both transport mechanisms with continuum models and compare them to experimental results. We show that electron diffusion can explain both the observed state-of-charge dependence and the time dependence. In contrast, we demonstrate that solvent diffusion can reproduce either the state-of-charge dependence or the time dependence of capacity fade. There is no intermediate regime where solvent diffusion can explain both dependencies simultaneously. Furthermore, we emphasize the crucial role of anode voltage and state-of-charge on SEI growth in general. Due to self-discharge, this dependence can explain deviations from the typical square-root behavior in the time domain. We conclude that electron diffusion is the relevant process leading to the state-of-charge dependent SEI growth. Further experiments are needed to investigate the reason for contributions to the capacity fade that are independent of the state-of-charge." @default.
- W4317937914 created "2023-01-25" @default.
- W4317937914 creator A5013132420 @default.
- W4317937914 creator A5020849015 @default.
- W4317937914 creator A5040582640 @default.
- W4317937914 date "2023-03-01" @default.
- W4317937914 modified "2023-10-14" @default.
- W4317937914 title "Growth of the solid-electrolyte interphase: Electron diffusion versus solvent diffusion" @default.
- W4317937914 cites W1970581450 @default.
- W4317937914 cites W1976543683 @default.
- W4317937914 cites W1977603059 @default.
- W4317937914 cites W1994484577 @default.
- W4317937914 cites W2017590852 @default.
- W4317937914 cites W2017908888 @default.
- W4317937914 cites W2029783496 @default.
- W4317937914 cites W2037447290 @default.
- W4317937914 cites W2037662406 @default.
- W4317937914 cites W2042581501 @default.
- W4317937914 cites W2048532212 @default.
- W4317937914 cites W2093650949 @default.
- W4317937914 cites W2098186059 @default.
- W4317937914 cites W2099314167 @default.
- W4317937914 cites W2117047946 @default.
- W4317937914 cites W2132414575 @default.
- W4317937914 cites W2152492366 @default.
- W4317937914 cites W2161600281 @default.
- W4317937914 cites W2256422229 @default.
- W4317937914 cites W2286746918 @default.
- W4317937914 cites W2312874713 @default.
- W4317937914 cites W2316283113 @default.
- W4317937914 cites W2331078757 @default.
- W4317937914 cites W2340971382 @default.
- W4317937914 cites W2432476102 @default.
- W4317937914 cites W2464273419 @default.
- W4317937914 cites W2527877831 @default.
- W4317937914 cites W2570584620 @default.
- W4317937914 cites W2608997523 @default.
- W4317937914 cites W2610497384 @default.
- W4317937914 cites W2622680715 @default.
- W4317937914 cites W2765279177 @default.
- W4317937914 cites W2767439356 @default.
- W4317937914 cites W2792330355 @default.
- W4317937914 cites W2792662281 @default.
- W4317937914 cites W2796282060 @default.
- W4317937914 cites W2916592458 @default.
- W4317937914 cites W2963013171 @default.
- W4317937914 cites W2974904579 @default.
- W4317937914 cites W2976289009 @default.
- W4317937914 cites W3014869563 @default.
- W4317937914 cites W3020697508 @default.
- W4317937914 cites W3098967086 @default.
- W4317937914 cites W3100495083 @default.
- W4317937914 cites W3123266717 @default.
- W4317937914 cites W3163914048 @default.
- W4317937914 cites W3196079175 @default.
- W4317937914 cites W4205652915 @default.
- W4317937914 cites W4206822378 @default.
- W4317937914 cites W4220968072 @default.
- W4317937914 cites W4280598508 @default.
- W4317937914 cites W4283069212 @default.
- W4317937914 doi "https://doi.org/10.1016/j.jpowsour.2023.232651" @default.
- W4317937914 hasPublicationYear "2023" @default.
- W4317937914 type Work @default.
- W4317937914 citedByCount "4" @default.
- W4317937914 countsByYear W43179379142023 @default.
- W4317937914 crossrefType "journal-article" @default.
- W4317937914 hasAuthorship W4317937914A5013132420 @default.
- W4317937914 hasAuthorship W4317937914A5020849015 @default.
- W4317937914 hasAuthorship W4317937914A5040582640 @default.
- W4317937914 hasBestOaLocation W43179379142 @default.
- W4317937914 hasConcept C121332964 @default.
- W4317937914 hasConcept C147120987 @default.
- W4317937914 hasConcept C147789679 @default.
- W4317937914 hasConcept C159467904 @default.
- W4317937914 hasConcept C17525397 @default.
- W4317937914 hasConcept C178790620 @default.
- W4317937914 hasConcept C185592680 @default.
- W4317937914 hasConcept C192562407 @default.
- W4317937914 hasConcept C2780471494 @default.
- W4317937914 hasConcept C62520636 @default.
- W4317937914 hasConcept C68801617 @default.
- W4317937914 hasConcept C69357855 @default.
- W4317937914 hasConcept C89395315 @default.
- W4317937914 hasConcept C97355855 @default.
- W4317937914 hasConceptScore W4317937914C121332964 @default.
- W4317937914 hasConceptScore W4317937914C147120987 @default.
- W4317937914 hasConceptScore W4317937914C147789679 @default.
- W4317937914 hasConceptScore W4317937914C159467904 @default.
- W4317937914 hasConceptScore W4317937914C17525397 @default.
- W4317937914 hasConceptScore W4317937914C178790620 @default.
- W4317937914 hasConceptScore W4317937914C185592680 @default.
- W4317937914 hasConceptScore W4317937914C192562407 @default.
- W4317937914 hasConceptScore W4317937914C2780471494 @default.
- W4317937914 hasConceptScore W4317937914C62520636 @default.
- W4317937914 hasConceptScore W4317937914C68801617 @default.
- W4317937914 hasConceptScore W4317937914C69357855 @default.
- W4317937914 hasConceptScore W4317937914C89395315 @default.
- W4317937914 hasConceptScore W4317937914C97355855 @default.