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- W4318766791 abstract "Abstract The combination of single-ion magnets (SIMs) and metal-organic frameworks (MOFs) is expected to produce new quantum materials. The principal issue to be solved in this regard is the development of new strategies for the synthesis of SIM-MOFs. This work demonstrates a new simple strategy for the synthesis of SIM-MOFs where a diamagnetic MOF is used as the framework into which the SIM sites are doped. 1 mol%, 0.5 mol%, and 0.2 mol% of the Co(II) ions are doped into the Zn(II) sites of [CH6N3][ZnII(HCOO)3]. The doped Co(II) sites in the MOFs perform as SIM with a positive D term of zero-field splitting. Temperature dependency of the relaxation time suggests suppressing spin- lattice relaxation by the rigid framework. Thus, this work represents a proof of concept for the creation of single-ion doped magnets in MOFs. This simple synthetic strategy will be widely applied for the creation of quantum magnetic materials." @default.
- W4318766791 created "2023-02-02" @default.
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- W4318766791 date "2023-02-01" @default.
- W4318766791 modified "2023-10-16" @default.
- W4318766791 title "Creation of Co(II) single-ion magnets by doping into Zn(II) diamagnetic metal-organic frameworks" @default.
- W4318766791 doi "https://doi.org/10.21203/rs.3.rs-2517253/v1" @default.
- W4318766791 hasPublicationYear "2023" @default.
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