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• W4319069441 abstract "Deep understanding of the chemical reaction and physical transport characteristics of 6-methyl-5-hepten-2-one (6-MHO) in different phases (e.g., skin, clothing) is important for modeling the indoor squalene/ozone reaction. In this study, we make the first attempt to accurately measure the physical transport parameters, i.e., the diffusion coefficient (Dm) and partition coefficient (K) of 6-MHO in different clothing (jeans, nylon, pure cotton T-shirt). A ventilated–airtight–ventilated testing procedure was designed, and relevant experiments were performed in 30 L small-scale chambers. The key parameters of 6-MHO (Dm and K) are determined by nonlinearly fitting the measured gas-phase concentration data with physical model using a hybrid optimization method. The high fitting accuracy (R2 > 0.93), good replication (relative deviations of determined Dm and K less than 16% for duplicated experiments), and further sensitivity analysis demonstrate the reliability and robustness of the method. In addition, the variation of the key parameters of 6-MHO in the pure cotton T-shirt with temperature (in the range of 20–37 °C) is investigated. Results indicate that Dm increases while K decreases with increasing temperature. This study provides some of the fundamental data for characterizing the squalene/ozone reaction and should be helpful for the subsequent dermal exposure in realistic indoor environments." @default.
• W4319069441 created "2023-02-04" @default.
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• W4319069441 date "2023-02-03" @default.
• W4319069441 modified "2023-10-17" @default.
• W4319069441 title "Measurement of the Diffusion and Partition Coefficients of 6-Methyl-5-hepten-2-one in Clothing" @default.
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• W4319069441 doi "https://doi.org/10.1021/acs.estlett.3c00024" @default.
• W4319069441 hasPublicationYear "2023" @default.
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