Matches in SemOpenAlex for { <https://semopenalex.org/work/W4319069538> ?p ?o ?g. }
- W4319069538 endingPage "119692" @default.
- W4319069538 startingPage "119692" @default.
- W4319069538 abstract "Pre-ozonation coagulation process had a very low and narrow range of ozone dosages for enhancing the dissolved organic matter (DOC) removal efficiency, in which over-oxidation may occur if the ozone dosage was not strictly controlled. In contrast, the proposed hybrid ozonation-coagulation (HOC) process with higher oxidation ability notably inhibited over-oxidation in this study, and exhibited improved DOC removal efficiency compared with coagulation at a much wider range of ozone dosages at different initial pH for the treatment of WWTP effluent. The HOC process also had a higher DOC removal efficiency than pre-ozonation coagulation. According to zeta potential analysis, a rising trend indicated that complexation between organic matter and metal coagulants persisted throughout the HOC process. However, the zeta potential remained almost unchanged during subsequent coagulation after pre-ozonation at high ozone dosages. Synchronous fluorescence spectroscopy analysis revealed that immediate entrapment and complexation between hydrolysed coagulants and oxidized intermediate organic matter occurred in the HOC process. Furthermore, FT-IR analysis showed that more oxygen-containing functional groups were generated, which were effectively trapped by metal coagulants and readily flocculated. To further prove the immediate entrapment and complexation during the HOC process, UPLC-Q-TOF-MS was applied to analyze the intermediate organic matter in the supernatant and flocs. The results implied that C21- organic matter was oxidized and decomposed into C11-C20, and C11-C20 intermediate organic matter was trapped and complexed by metal coagulants once formed, which led to the increase of C11-C20 in the flocs. Nevertheless, the catalytic ozonation process (γ-Al2O3/O3) with the same oxidation ability as the HOC process decomposed the organic matter into C1-C10. XPS analysis further confirmed the immediate entrapment and removal of aliphatic/aromatic carbon and oxygen-containing functional groups during the HOC process. Therefore, over-oxidation can be effectively inhibited, and wide range of ozone dosages was obtained during the HOC process, which facilitate the application of the HOC process." @default.
- W4319069538 created "2023-02-04" @default.
- W4319069538 creator A5003369960 @default.
- W4319069538 creator A5023578096 @default.
- W4319069538 creator A5033666227 @default.
- W4319069538 creator A5037817783 @default.
- W4319069538 creator A5052195787 @default.
- W4319069538 creator A5057837748 @default.
- W4319069538 creator A5074354869 @default.
- W4319069538 creator A5075380979 @default.
- W4319069538 creator A5075943675 @default.
- W4319069538 creator A5077700424 @default.
- W4319069538 creator A5090584158 @default.
- W4319069538 date "2023-04-01" @default.
- W4319069538 modified "2023-10-15" @default.
- W4319069538 title "Unraveling the over-oxidation inhibition mechanism during the hybrid ozonation-coagulation process: Immediate entrapment and complexation between intermediate organic matter and coagulants" @default.
- W4319069538 cites W1806194750 @default.
- W4319069538 cites W1987120408 @default.
- W4319069538 cites W1999880283 @default.
- W4319069538 cites W2000235668 @default.
- W4319069538 cites W2014485479 @default.
- W4319069538 cites W2026585492 @default.
- W4319069538 cites W2029358844 @default.
- W4319069538 cites W2044781364 @default.
- W4319069538 cites W2052534919 @default.
- W4319069538 cites W2058900788 @default.
- W4319069538 cites W2065753825 @default.
- W4319069538 cites W2071667883 @default.
- W4319069538 cites W2072559578 @default.
- W4319069538 cites W2077329198 @default.
- W4319069538 cites W2174601685 @default.
- W4319069538 cites W2327712807 @default.
- W4319069538 cites W2345815996 @default.
- W4319069538 cites W2565294887 @default.
- W4319069538 cites W2565874714 @default.
- W4319069538 cites W2569933389 @default.
- W4319069538 cites W2588016605 @default.
- W4319069538 cites W2700156820 @default.
- W4319069538 cites W2765995478 @default.
- W4319069538 cites W2781055474 @default.
- W4319069538 cites W2883481668 @default.
- W4319069538 cites W2899761915 @default.
- W4319069538 cites W2926821521 @default.
- W4319069538 cites W2944588903 @default.
- W4319069538 cites W2952468984 @default.
- W4319069538 cites W2999762075 @default.
- W4319069538 cites W3011491184 @default.
- W4319069538 cites W3016135648 @default.
- W4319069538 cites W3033145958 @default.
- W4319069538 cites W3087739769 @default.
- W4319069538 cites W3121342607 @default.
- W4319069538 cites W3158880406 @default.
- W4319069538 cites W3175636197 @default.
- W4319069538 cites W3197587177 @default.
- W4319069538 cites W3204268612 @default.
- W4319069538 cites W4200216526 @default.
- W4319069538 cites W4210698394 @default.
- W4319069538 cites W4210851622 @default.
- W4319069538 cites W4220750786 @default.
- W4319069538 cites W4280597118 @default.
- W4319069538 cites W4281769168 @default.
- W4319069538 doi "https://doi.org/10.1016/j.watres.2023.119692" @default.
- W4319069538 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36758355" @default.
- W4319069538 hasPublicationYear "2023" @default.
- W4319069538 type Work @default.
- W4319069538 citedByCount "3" @default.
- W4319069538 countsByYear W43190695382023 @default.
- W4319069538 crossrefType "journal-article" @default.
- W4319069538 hasAuthorship W4319069538A5003369960 @default.
- W4319069538 hasAuthorship W4319069538A5023578096 @default.
- W4319069538 hasAuthorship W4319069538A5033666227 @default.
- W4319069538 hasAuthorship W4319069538A5037817783 @default.
- W4319069538 hasAuthorship W4319069538A5052195787 @default.
- W4319069538 hasAuthorship W4319069538A5057837748 @default.
- W4319069538 hasAuthorship W4319069538A5074354869 @default.
- W4319069538 hasAuthorship W4319069538A5075380979 @default.
- W4319069538 hasAuthorship W4319069538A5075943675 @default.
- W4319069538 hasAuthorship W4319069538A5077700424 @default.
- W4319069538 hasAuthorship W4319069538A5090584158 @default.
- W4319069538 hasConcept C107872376 @default.
- W4319069538 hasConcept C118552586 @default.
- W4319069538 hasConcept C127413603 @default.
- W4319069538 hasConcept C147455438 @default.
- W4319069538 hasConcept C148815931 @default.
- W4319069538 hasConcept C155672457 @default.
- W4319069538 hasConcept C15744967 @default.
- W4319069538 hasConcept C178790620 @default.
- W4319069538 hasConcept C179104552 @default.
- W4319069538 hasConcept C185592680 @default.
- W4319069538 hasConcept C2778382381 @default.
- W4319069538 hasConcept C42360764 @default.
- W4319069538 hasConcept C48743137 @default.
- W4319069538 hasConcept C508106653 @default.
- W4319069538 hasConcept C86181022 @default.
- W4319069538 hasConcept C87717796 @default.
- W4319069538 hasConceptScore W4319069538C107872376 @default.
- W4319069538 hasConceptScore W4319069538C118552586 @default.
- W4319069538 hasConceptScore W4319069538C127413603 @default.