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- W4319315907 abstract "Abstract Two‐dimensional (2D) materials catalysts provide an atomic‐scale view on a fascinating arena for understanding the mechanism of electrocatalytic carbon dioxide reduction (CO 2 ECR). Here, we successfully exfoliated both layered and nonlayered ultra‐thin metal phosphorous trichalcogenides (MPCh 3 ) nanosheets via wet grinding exfoliation (WGE), and systematically investigated the mechanism of MPCh 3 as catalysts for CO 2 ECR. Unlike the layered CoPS 3 and NiPS 3 nanosheets, the active Sn atoms tend to be exposed on the surfaces of nonlayered SnPS 3 nanosheets. Correspondingly, the nonlayered SnPS 3 nanosheets exhibit clearly improved catalytic activity, showing formic acid selectivity up to 31.6 % with −7.51 mA cm −2 at −0.65 V vs. RHE. The enhanced catalytic performance can be attributed to the formation of HCOO* via the first proton‐electron pair addition on the SnPS 3 surface. These results provide a new avenue to understand the novel CO 2 ECR mechanism of Sn‐based and MPCh 3 ‐based catalysts." @default.
- W4319315907 created "2023-02-08" @default.
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- W4319315907 date "2023-02-27" @default.
- W4319315907 modified "2023-10-17" @default.
- W4319315907 title "Exfoliated 2D Layered and Nonlayered Metal Phosphorous Trichalcogenides Nanosheets as Promising Electrocatalysts for CO<sub>2</sub> Reduction" @default.
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- W4319315907 doi "https://doi.org/10.1002/ange.202217253" @default.
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