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- W4319661808 endingPage "119725" @default.
- W4319661808 startingPage "119725" @default.
- W4319661808 abstract "Developing high-performance catalytic systems for eliminating contaminants effectively in water has received a lot of attention. However, the complexity of practical wastewater poses a challenge for degrading organic pollutants. Non-radical active species with strong resistance to interference have shown great advantages in degrading organic pollutants under complex aqueous conditions. Herein, a novel system was constructed by Fe(dpa)Cl2 (FeL, dpa = N, N'-(4-nitro-1,2-phenylene) dipicolinamide) activating peroxymonosulfate (PMS). The mechanism study verified that the FeL/PMS system had high efficiency in producing high-valent iron-oxo and singlet oxygen (1O2) to degrade various organic pollutants. In addition, the chemical bonding between PMS and FeL was elucidated by the density functional theory (DFT) calculations. The FeL/PMS system could remove 96% Reactive Red 195 (RR195) in 2 min, which was much higher than other systems involved in this study. More attractively, the FeL/PMS system demonstrated general resistance to interference from common anions (Cl−, HCO3−, NO3− and SO42−), humic acid (HA) and pH changes and were thus compatible with various natural waters. This work provides a new approach for producing non-radical active species, which is a promising catalytic system for water treatment." @default.
- W4319661808 created "2023-02-10" @default.
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- W4319661808 date "2023-04-01" @default.
- W4319661808 modified "2023-10-11" @default.
- W4319661808 title "Rapid activation of peroxymonosulfate with iron(Ⅲ) complex for organic pollutants degradation via a non-radical pathway" @default.
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- W4319661808 doi "https://doi.org/10.1016/j.watres.2023.119725" @default.
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