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• W4319832247 abstract "Abstract The reactivity of alkynylphosphines with Lewis acidic boranes has been well established in recent years thanks to the advent of frustrated Lewis pairs (FLPs), often leading to a 1,1‐carboboration reaction and the formation of an intramolecular phosphinoborane FLP. Our group recently discovered that introduction of an ionizable group in the γ‐position of an alkynylphosphine result in an unexpected rearrangement reaction to yield zwitterionic allenic‐phosphonium borate products which are produced via a transient 3‐coordinate phosphonium allenylidene. Herein, we describe how substituent effects on the γ‐carbon impact this reactivity and explore how bis(alkynyl)phosphines behave under similar reaction conditions." @default.
• W4319832247 created "2023-02-11" @default.
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• W4319832247 date "2023-01-23" @default.
• W4319832247 modified "2023-09-26" @default.
• W4319832247 title "Reactivity of Alkynyl Phosphines with Lewis Acids for the Synthesis of Allenic Phosphonium Borate Zwitterions" @default.
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• W4319832247 doi "https://doi.org/10.1002/zaac.202200383" @default.
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