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- W4320000092 abstract "Currently, the smartest way for solving this environmental issue is the-inspired-by-nature method, which is an artificially-photoassisted conversion of CO2 into chemicals, fuels, and energy. Some systems for such conversion include photovoltaic (PV)-electrocatalysis, photoelectrode thin films, photocatalyst particle suspensions, carbon capture and sequestration, CO2 injection for oil recovery, and converting CO2 into dry ice. However, despite advances in the mechanism of reducing CO2 with a single-electron system, the reduction and oxidation pathways, and identity of the redox species remain elusive. This is viewed in perspective, considering the extensive research on selecting suitable photocatalysts for converting solar light to charge-carriers in the redox reactions since the first report of CO2 reduction in 1979. Amongst the numerous semiconducting materials, e.g., C3N4, CdS, Cu2O, and TiO2, perovskite-based nanomaterials are the most promising for CO2 reduction. This is because these materials possess large charge-carrier motility, high light-harvesting activities, and compositional flexibility. The latter facilitates an appreciable bandgap for absorbing a wide spectrum of solar light, low exciton binding energy, longer exciton diffusion length, and easily tunable bandgap. The chapter also summarizes the factors such as heterojunction construction, structural formation, overlayer modification, defects engineering, etc., that are essential for enhancing selectivity and productivity." @default.
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- W4320000092 date "2023-01-01" @default.
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- W4320000092 title "Perovskite-based nanomaterials for CO2 conversion" @default.
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- W4320000092 doi "https://doi.org/10.1016/b978-0-323-89851-5.00004-4" @default.
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