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- W4320032888 abstract "Herein, a twisty C-TiO2/PCN (CNT) Step-scheme (S-scheme) heterojunction is fabricated and applied to degrade ciprofloxacin (CIP) with the assistance of ultrasonic vibration and visible light irradiation. The nitrogen-rich twisty polymeric carbon nitride (PCN) can not only induce a non-centrosymmetric structure with enhanced polarity for a better piezoelectric effect but also provide abundant lone pair electrons to promote n→π* transition during photocatalysis. Its hybridization with C-TiO2 particles can construct S-scheme heterojunction in CNT. During the piezo-photocatalysis, the strain-induced polarization electric field in the heterojunction can regulate the electron migration between the two components, resulting in a more effective CIP degradation. With the synergistic effect of ultrasonic vibration and visible light irradiation, the reaction rate constant of CIP degradation by CNT increases to 0.0517 min−1, which is 1.86 times that of photocatalysis and 6.46 times that of ultrasound. This system exhibits a stable CIP decomposition efficiency under the interference of various environmental factors. In addition, the in-depth investigation found that three pathways and 12 major intermediates with reduced toxicity are produced after the reaction. Hopefully, the construction of this twisty CNT S-scheme heterojunction with enhanced piezo-photocatalytic effect offers inspiration for the design of environmentally functional materials." @default.
- W4320032888 created "2023-02-12" @default.
- W4320032888 creator A5005113512 @default.
- W4320032888 creator A5013262195 @default.
- W4320032888 creator A5016825131 @default.
- W4320032888 creator A5056452538 @default.
- W4320032888 creator A5058150270 @default.
- W4320032888 creator A5072419737 @default.
- W4320032888 creator A5078425193 @default.
- W4320032888 creator A5086031269 @default.
- W4320032888 date "2023-02-11" @default.
- W4320032888 modified "2023-10-17" @default.
- W4320032888 title "Twisty C‐TiO <sub>2</sub> /PCN S‐Scheme Heterojunction with Enhanced n→π * Electronic Excitation for Promoted Piezo‐Photocatalytic Effect" @default.
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