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- W4320170181 abstract "The fluorescence-based temperature measurement technology based on rare earth doped NaBiF4 matrix luminescent materials has aroused great interest. However, most of the current works depend on the thermal coupling energy levels obtained from a single luminous center Er3+or Tm3+ in the NaBiF4 matrix. Additionally, the energy gap ΔE (200-2000 cm−1) of the thermally coupled levels (TCLs) limits the sensitivity and accuracy of temperature measuring materials to be improved. Here, we propose to prepare Yb3+/Er3+/Tm3+ triple doped NaBiF4 nanomaterials and use Arrhenius equation to break TCL's energy gap (ΔE) restriction based on the non-thermally coupled levels (NTCLs) of the double luminous centers Er3+ and Tm3+. The higher temperature sensitivity and the lower temperature uncertainty based on NTCLs of fluorescence intensity ratio (NTCLs-FIR) are confirmed, which is compared with the temperature sensitivity based on TCLs-FIR. Simultaneously, the crystal structure, morphology, photoluminescence properties, especially the photoluminescence mechanism and energy transfer of Yb3+/Er3+/Tm3+ doped NaBiF4 nanomaterials are evaluated. This study provides a new insight into integrating Yb3+/Er3+/Tm3+ triple doped single NaBiF4 matrix luminescent materials into optical thermometric materials using FIR technology." @default.
- W4320170181 created "2023-02-13" @default.
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- W4320170181 date "2023-05-01" @default.
- W4320170181 modified "2023-10-06" @default.
- W4320170181 title "Temperature-responsive NaBiF4:Yb3+, Er3+/Tm3+ based on non-thermally coupled levels" @default.
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- W4320170181 doi "https://doi.org/10.1016/j.jlumin.2023.119711" @default.
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