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- W4320476422 abstract "Broadband optical response and strong optical nonlinearity have enabled MXenes to be applied in numerous ultrafast photonic devices. Here, we explored the nonlinear optical properties of a novel MXene, Ta2C, and demonstrated a femtosecond fiber laser with a Ta2C-based saturable absorber (SA). First-principles calculations were employed to fully reveal the structural and electronic properties of the Ta2C MXene. The third-order nonlinear optical properties of the as-prepared Ta2C nanosheets were measured from the visible to near-infrared regime by the commonly used open-aperture Z-scan technique. Its maximum nonlinear absorption coefficient was fitted to be −0.42 cm/GW, implying its broad application prospects in nonlinear photonic devices. Moreover, Ta2C MXene-coated microfibers as SAs were integrated into erbium-doped fiber laser cavities. Long-term stable mode-locked pulses centered at 1560.1 nm were generated by the constructed laser device. The ultrashort pulse duration of about 774 fs and high signal-to-noise ratio of over 50 dB indicate that Ta2C MXene is a promising material for generating ultrafast pulses." @default.
- W4320476422 created "2023-02-14" @default.
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- W4320476422 date "2023-06-01" @default.
- W4320476422 modified "2023-10-16" @default.
- W4320476422 title "Ta2C MXene: Nonlinear optical properties and application in femtosecond fiber laser" @default.
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- W4320476422 doi "https://doi.org/10.1016/j.optlastec.2023.109178" @default.
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