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• W4320717329 abstract "The combination of asymmetric organocatalysis with the (pseudo)-halogen effect enables the formation of chiral norcarane scaffolds in high yields and selectivities (up to 92% yield, >99% ee, and >95:5 d.r.). This was achieved by reacting (pseudo)-halogenated 3-vinyl chromones with in situ generated chiral dienamines in an inverse electron demand [4 + 2] cycloaddition followed by an intramolecular SN2 reaction. These scaffolds could easily undergo photoinduced rearrangements or lactonization to form intricate chiral ring structures." @default.
• W4320717329 created "2023-02-15" @default.
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• W4320717329 date "2023-02-14" @default.
• W4320717329 modified "2023-09-27" @default.
• W4320717329 title "Asymmetric Organocatalyzed Cascade Reactions─Merging the <i>pseudo</i>-Halogen and Halogen Effect with Dienamine Catalysis" @default.
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• W4320717329 doi "https://doi.org/10.1021/acs.orglett.3c00220" @default.
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