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- W4320921217 abstract "Abstract Ethanol has been used as a renewable hydrogen‐donor in the conversion of a lignin model molecule in subcritical conditions. Noble metal‐free porous mixed oxides, obtained by activation of Cu−Ni−Al and Cu−Ni−Fe layered double hydroxide (LDH) precursors, have been used as heterogeneous catalysts for Meerwein‐Ponndorf‐Verley (MPV) hydrogen transfer and further hydrogenation by ethanol dehydrogenation products. Both the Cu/(Cu+Ni) ratio and the nature of the trivalent cation (Al or Fe) affect the activity of the catalysts, as well as the selectivity towards the different steps of the hydrogenation reactions and the cleavage of lignin‐like phenylether bonds. Accounting for the peculiar behaviour of Cu 2+ and M(III) cations in the synthesis of LDHs, the coprecipitation of the precursors has been monitored by titration experiments. Structural and textural properties of the catalysts are closely related to the composition of the LDH precursors." @default.
- W4320921217 created "2023-02-16" @default.
- W4320921217 creator A5008552432 @default.
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- W4320921217 creator A5090942529 @default.
- W4320921217 date "2023-02-28" @default.
- W4320921217 modified "2023-10-02" @default.
- W4320921217 title "Design of Multicationic Copper‐Bearing Layered Double Hydroxides for Catalytic Application in Biorefinery" @default.
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