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- W4320921981 abstract "The prototypical drug carrier [CoII(L1)Cl]PF6 (1), where L1 is a tripodal amine bound to pyridine and methyl-imidazoles, had its electrocatalytic water splitting activity studied under different pH conditions. This species contains a high-spin 3d7 CoII metal center, and is capable of generating both H2 from water reduction and O2 from water oxidation. Turnover numbers reach 390 after 3 h for water reduction. Initial water oxidation activity is molecular, with TONs of 71 at pH 7 and 103 at pH 11.5. The results reveal that species 1 can undergo several redox transformations, including reduction to the 3d8 CoI species that precedes a LS3d6 hydride for water reduction, as well as nominal CoIVO and CoIII-OOH species required for water oxidation. Post-catalytic analyses confirm the molecular nature of reduction and support initial molecular activity for oxidation." @default.
- W4320921981 created "2023-02-16" @default.
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- W4320921981 date "2023-05-01" @default.
- W4320921981 modified "2023-10-16" @default.
- W4320921981 title "A bioinspired cobalt catalyst based on a tripodal imidazole/pyridine platform capable of water reduction and oxidation" @default.
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- W4320921981 doi "https://doi.org/10.1016/j.jinorgbio.2023.112162" @default.
- W4320921981 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36841008" @default.
- W4320921981 hasPublicationYear "2023" @default.
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