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• W4320922016 abstract "In steam reforming of organics in a fixed-bed reactor, catalyst particles in varied location of catalyst bed will experience different history of contacting with reactants/products. This may affect accumulation of coke in varied section of catalyst bed, which are investigated in steam reforming of some typical oxygen-containing organics (acetic acid, acetone and ethanol) and hydrocarbons (n-hexane and toluene) in a fixed-bed reactor with double layers of catalyst bed for investigating coking depth at 650 °C over Ni/KIT-6 catalyst in this study. The results indicated that the intermediates derived from the oxygen-containing organics in steam reforming could hardly penetrate the upper-layer catalyst to form coke in the lower-layer catalyst. In converse, they reacted quickly over the upper-layer catalyst via gasification or coking, forming coke almost exclusively in the upper-layer catalyst. The hydrocarbon intermediates from the dissociation of hexane or toluene could easily penetrate and reach the lower-layer catalyst to form even more coke therein than the upper-layer catalyst. The characterization showed that the insufficient gasification of *CxHy species led to their aggregation/integration to form more aromatic coke, especially from n-hexane. The aromatic-ring containing intermediates from toluene tended to integrate with *OH species to form ketones that further involved in coking, forming coke of less aromatic nature than that from n-hexane. Steam reforming of oxygen-containing organics also produced oxygen-containing intermediates and coke of higher aliphatic nature, lower carbon to hydrogen (C/H) ratio, lower crystallinity and thermal stability." @default.
• W4320922016 created "2023-02-16" @default.
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• W4320922016 date "2023-06-01" @default.
• W4320922016 modified "2023-10-02" @default.
• W4320922016 title "Distinct coking depth in steam reforming of oxygen-containing organics and hydrocarbons" @default.
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• W4320922016 doi "https://doi.org/10.1016/j.jcis.2023.02.070" @default.
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