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- W4321004412 abstract "Abstract The poor stability of Ru-based acidic oxygen evolution (OER) electrocatalysts has greatly hampered their application in polymer electrolyte membrane electrolyzers (PEMWEs). Traditional understanding of performance degradation centered on influence of bias fails in describing the stability trend, calling for deep dive into the essential origin of inactivation. Here we uncover the decisive role of reaction route (including catalytic mechanism and intermediates binding strength) on operational stability of Ru-based catalysts. Using MRuO x (M = Ce 4+ , Sn 4+ , Ru 4+ , Cr 4+ ) solid solution as structure model, we find the reaction route, thereby stability, can be customized by controlling the Ru charge. The screened SnRuO x thus exhibits orders of magnitude lifespan extension. A scalable PEMWE single cell using SnRuO x anode conveys an ever-smallest degradation rate of 53 μV h −1 during a 1300 h operation at 1 A cm −2 ." @default.
- W4321004412 created "2023-02-17" @default.
- W4321004412 creator A5020188233 @default.
- W4321004412 creator A5022930741 @default.
- W4321004412 creator A5023582873 @default.
- W4321004412 creator A5025068432 @default.
- W4321004412 creator A5025627244 @default.
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- W4321004412 creator A5038741162 @default.
- W4321004412 creator A5041883522 @default.
- W4321004412 creator A5045370357 @default.
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- W4321004412 creator A5060978357 @default.
- W4321004412 creator A5064803348 @default.
- W4321004412 creator A5078526337 @default.
- W4321004412 date "2023-02-15" @default.
- W4321004412 modified "2023-10-16" @default.
- W4321004412 title "Customized reaction route for ruthenium oxide towards stabilized water oxidation in high-performance PEM electrolyzers" @default.
- W4321004412 cites W1623117034 @default.
- W4321004412 cites W1970127494 @default.
- W4321004412 cites W1974980751 @default.
- W4321004412 cites W2002145988 @default.
- W4321004412 cites W2007395042 @default.
- W4321004412 cites W2016734948 @default.
- W4321004412 cites W2020007931 @default.
- W4321004412 cites W2027329930 @default.
- W4321004412 cites W2028549346 @default.
- W4321004412 cites W2031803642 @default.
- W4321004412 cites W2033140097 @default.
- W4321004412 cites W2036113194 @default.
- W4321004412 cites W2063714883 @default.
- W4321004412 cites W2079105963 @default.
- W4321004412 cites W2083222334 @default.
- W4321004412 cites W2087698390 @default.
- W4321004412 cites W2116419646 @default.
- W4321004412 cites W2133406747 @default.
- W4321004412 cites W2145388151 @default.
- W4321004412 cites W2167590372 @default.
- W4321004412 cites W2270001164 @default.
- W4321004412 cites W2310142985 @default.
- W4321004412 cites W2317238370 @default.
- W4321004412 cites W2318269538 @default.
- W4321004412 cites W2415833664 @default.
- W4321004412 cites W2465590178 @default.
- W4321004412 cites W2514157351 @default.
- W4321004412 cites W2547752795 @default.
- W4321004412 cites W2571310289 @default.
- W4321004412 cites W2576668085 @default.
- W4321004412 cites W2587375637 @default.
- W4321004412 cites W2591036596 @default.
- W4321004412 cites W2597561719 @default.
- W4321004412 cites W2597898713 @default.
- W4321004412 cites W2604583515 @default.
- W4321004412 cites W2740568941 @default.
- W4321004412 cites W2756200386 @default.
- W4321004412 cites W2765466599 @default.
- W4321004412 cites W2767331214 @default.
- W4321004412 cites W2768954979 @default.
- W4321004412 cites W2772586412 @default.
- W4321004412 cites W2805591174 @default.
- W4321004412 cites W2807304377 @default.
- W4321004412 cites W2810958890 @default.
- W4321004412 cites W2885548404 @default.
- W4321004412 cites W2894888152 @default.
- W4321004412 cites W2910372448 @default.
- W4321004412 cites W2911036998 @default.
- W4321004412 cites W2917007993 @default.
- W4321004412 cites W2922366141 @default.
- W4321004412 cites W2923580268 @default.
- W4321004412 cites W2940789693 @default.
- W4321004412 cites W2950573241 @default.
- W4321004412 cites W2969273688 @default.
- W4321004412 cites W2971489451 @default.
- W4321004412 cites W2981608441 @default.
- W4321004412 cites W2991545587 @default.
- W4321004412 cites W2992689825 @default.
- W4321004412 cites W2996204627 @default.
- W4321004412 cites W2997985037 @default.
- W4321004412 cites W2999583776 @default.
- W4321004412 cites W3004296233 @default.
- W4321004412 cites W3005611682 @default.
- W4321004412 cites W3006713606 @default.
- W4321004412 cites W3009722102 @default.
- W4321004412 cites W3013643556 @default.
- W4321004412 cites W3020542478 @default.
- W4321004412 cites W3023846881 @default.
- W4321004412 cites W3034001092 @default.
- W4321004412 cites W3044917208 @default.
- W4321004412 cites W3045404961 @default.
- W4321004412 cites W3048453303 @default.
- W4321004412 cites W3087041690 @default.
- W4321004412 cites W3090555410 @default.
- W4321004412 cites W3090865632 @default.
- W4321004412 cites W3093851524 @default.
- W4321004412 cites W3094173475 @default.
- W4321004412 cites W3100410888 @default.
- W4321004412 cites W3100475594 @default.
- W4321004412 cites W3106197836 @default.
- W4321004412 cites W3120716797 @default.