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- W4321439057 endingPage "142031" @default.
- W4321439057 startingPage "142031" @default.
- W4321439057 abstract "Lithium-sulfur (Li-S) battery has been recognized as a new energy storage device with broad prospects because of its satisfactory specific capacity and theoretical energy density. Nevertheless, the shuttle effect of polysulfides seriously hinders the real applications of high-sulfur-loaded Li-S batteries. To remove the hurdle, hierarchical lamellar single-walled carbon nanotube aerogels (SWCNTAs) are herein fabricated and applied as multifunctional interlayers in Li-S batteries, which exhibit an initial area-specific capacity as high as 7.1 mAh cm−2 at a sulfur loading of 8.02 mg cm−2. The introduced SWCNTA interlayers can lower the internal resistance and suppress the shuttling of polysulfides by a layer-by-layer physical blocking mechanism. Moreover, owing to the super wettability of SWCNTAs, electrolytes with a dosage of 10 μL mg−1 could effectively wet and infiltrate the interlayers, rendering the lean-electrolyte Li-S batteries a high specific capacity of 559 mAh g−1 at a sulfur loading of 10.35 mg cm−2 after 60 cycles. This work presents an example for rationally designing the interlayers structures for high-sulfur loading batteries, which paves a stepping stone for the future commercialization of Li-S batteries." @default.
- W4321439057 created "2023-02-22" @default.
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- W4321439057 date "2023-04-01" @default.
- W4321439057 modified "2023-10-15" @default.
- W4321439057 title "Hierarchical lamellar single-walled carbon nanotube aerogel interlayers for stable lithium-sulfur batteries with high-sulfur-loading" @default.
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- W4321439057 doi "https://doi.org/10.1016/j.cej.2023.142031" @default.
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