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- W4321460416 abstract "In the context of catalysis, the optimal catalyst support structures should possess both high surface area and low mass transport resistance, and porous structures composed of micropores with additionally processed channels happen to meet both features. An open-source pore network modeling package, OpenPNM, was used to investigate the advection diffusion reaction process in such hierarchy porous media. Validation was performed via comparisons to the results obtained from the commercial finite element solver, COMSOL. It is shown that pore network modeling can satisfactorily simulate the reactive transport in pores media with a first order reaction kinetics. Under a wide range of local Peclet numbers (from close to 0 to about 10), the maximal relative error of local concentration concerning the finite element results is about 15.7%. Compared with the scenario where there are no additional channels, these channels can dramatically enhance the mass transport. A multi-channel featured porous system can be the desirable structure for catalyst application, and the optimized structural parameters were given." @default.
- W4321460416 created "2023-02-22" @default.
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- W4321460416 date "2023-05-01" @default.
- W4321460416 modified "2023-10-15" @default.
- W4321460416 title "Pore network modeling of advection-diffusion-reaction in porous media: The effects of channels" @default.
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- W4321460416 doi "https://doi.org/10.1016/j.ces.2023.118577" @default.
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