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• W4321481567 abstract "We perform magnetization sweeps on the high-performing single-molecule magnet [Dy(Cpttt)2][B(C6F5)4] (Cpttt = C5H2tBu3-1,2,4; tBu = C(CH3)3) to determine the quantum tunneling gap of the ground-state avoided crossing at zero-field, finding a value on the order of 10-7 cm-1. In addition to the pure crystalline material, we also measure the tunnel splitting of [Dy(Cpttt)2][B(C6F5)4] dissolved in dichloromethane (DCM) and 1,2-difluorobenzene (DFB). We find that concentrations of 200 or 100 mM [Dy(Cpttt)2][B(C6F5)4] in these solvents increases the size of the tunneling gap compared to the pure sample, despite a similarity in the strength of the dipolar fields, indicating that either a structural or vibrational change due to the environment increases quantum tunneling rates." @default.
• W4321481567 created "2023-02-23" @default.
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• W4321481567 date "2023-02-22" @default.
• W4321481567 modified "2023-10-13" @default.
• W4321481567 title "Measurement of the Quantum Tunneling Gap in a Dysprosocenium Single-Molecule Magnet" @default.
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• W4321481567 doi "https://doi.org/10.1021/acs.jpclett.3c00034" @default.
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