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• W4322617020 endingPage "5094" @default.
• W4322617020 startingPage "5083" @default.
• W4322617020 abstract "High-potential Mn3+/Mn2+ redox couple (>1.3 V vs SHE) in a static battery system is rarely reported due to the shuttle and disproportionation of Mn3+ in aqueous solutions. Herein, based on reversible stripping/plating of the Sn anode and stabilized Mn2+/Mn3+ redox couple in the cathode, an aqueous Sn-Mn full battery is established in acidic electrolytes. Sn anode exhibits high deposition efficiency, low polarization, and excellent stability in acidic electrolytes. With the help of H+ and a complexing agent, a reversible conversion between Mn2+ and Mn3+ ions takes place on the graphite surface. Pyrophosphate ligand is initially employed to form a protective layer through a complexation process with Sn4+ on the electrode surface, effectively preventing Mn3+ from disproportionation and hindering the uncontrollable diffusion of Mn3+ to electrolytes. Benefiting from the rational design, the full battery delivers satisfied electrochemical performance including a large capacity (0.45 mAh cm-2 at 5 mA cm-2), high discharge plateau voltage (>1.6 V), excellent rate capability (58% retention from 5 to 30 mA cm-2), and superior cycling stability (no decay after 30 000 cycles). The battery design strategy realizes a robustly stable Mn3+/Mn2+ redox reaction, which broadens research into ultrafast acidic battery systems." @default.
• W4322617020 created "2023-03-01" @default.
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• W4322617020 date "2023-02-28" @default.
• W4322617020 modified "2023-10-16" @default.
• W4322617020 title "A Static Tin–Manganese Battery with 30000-Cycle Lifespan Based on Stabilized Mn³⁺/Mn²⁺ Redox Chemistry" @default.
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• W4322617020 doi "https://doi.org/10.1021/acsnano.3c00242" @default.
• W4322617020 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36853201" @default.
• W4322617020 hasPublicationYear "2023" @default.
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