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- W4322719641 abstract "A cathode substrate with strong adsorption of lithium polysulfides (LiPSs) has been preferred for lithium-sulfur (Li-S) batteries. However, the recent finding that controlled growth of lithium sulfides (Li2 S) during discharge is crucial for S utilization stimulates improvement of this preference. Here, the Li2 S growth and cell capacity in the LiPS binding energy landscape of cathode substrates are investigated. Specifically, Co-based ternary oxides are employed to obtain binding energies in the range of 4.0-7.4 eV. Of these substrates, only the MnCo2 O4 substrate with moderate LiPS affinity exhibits 3D Li2 S growth. The MnCo2 O4 cells achieve high sulfur utilization up to 84% at 0.2 C and excellent performance even under high sulfur loading/lean electrolyte conditions. In contrast, weak affinity substrates such as ZnCo2 O4 and strong affinity substrates such as NiCo2 O4 and CuCo2 O4 exhibit low discharge capacity with 2D Li2 S growth. For optimal LiPS affinity driving 3D growth, a balance between promoting LiPS adsorption and diffusion limitation in the LiPS adsorption layer is suggested." @default.
- W4322719641 created "2023-03-03" @default.
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- W4322719641 date "2023-03-01" @default.
- W4322719641 modified "2023-10-08" @default.
- W4322719641 title "The Polysulfide‐Cathode Binding Energy Landscape for Lithium Sulfide Growth in Lithium‐Sulfur Batteries" @default.
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- W4322719641 doi "https://doi.org/10.1002/advs.202206057" @default.
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