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• W4322753611 abstract "A photocatalyst TiO2 /Ti-BPDC-Pt is developed with a self-grown TiO2 /Ti-metal-organic framework (MOF) heterojunction, i.e., TiO2 /Ti-BPDC, and selectively anchored high-density Pt single-atomic cocatalysts on Ti-BPDC for photocatalytic hydrogen evolution. This intimate heterojunction, growing from the surface pyrolytic reconstruction of Ti-BPDC, works in a direct Z-scheme, efficiently separating electrons and holes. Pt is selectively anchored on Ti-BPDC by ligands and is found in the form of single atoms with loading up to 1.8 wt %. The selective location of Pt is the electron-enriched domain of the heterojunction, which further enhances the utilization of the separated electrons. This tailored TiO2 /Ti-BPDC-Pt shows a significantly enhanced activity of 12.4 mmol g-1 h-1 compared to other TiO2 - or MOF-based catalysts. The structure-activity relationship further proves the balance of two simultaneously exposed domains of heterojunctions is critical to fulfilling this kind of catalyst." @default.
• W4322753611 created "2023-03-03" @default.
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• W4322753611 date "2023-04-03" @default.
• W4322753611 modified "2023-09-30" @default.
• W4322753611 title "Engineering a Self‐Grown TiO₂/Ti‐MOF Heterojunction with Selectively Anchored High‐Density Pt Single‐Atomic Cocatalysts for Efficient Visible‐Light‐Driven Hydrogen Evolution" @default.
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• W4322753611 doi "https://doi.org/10.1002/anie.202217439" @default.
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