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• W4322758226 abstract "The local coordination environment of catalytical moieties directly determines the performance of electrochemical energy storage and conversion devices, such as Li-O2 batteries (LOBs) cathode. However, understanding how the coordinative structure affects the performance, especially for non-metal system, is still insufficient. Herein, a strategy that introduces S-anion to tailor the electronic structure of nitrogen-carbon catalyst (SNC) is proposed to improve the LOBs performance. This study unveils that the introduced S-anion effectively manipulates the p-band center of pyridinic-N moiety, substantially reducing the battery overpotential by accelerating the generation and decomposition of intermediate products Li1-3 O4 . The lower adsorption energy of discharging product Li2 O2 on NS pair accounts for the long-term cyclic stability by exposing the high active area under operation condition. This work demonstrates an encouraging strategy to enhance LOBs performance by modulating the p-band center on non-metal active sites." @default.
• W4322758226 created "2023-03-03" @default.
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• W4322758226 date "2023-03-02" @default.
• W4322758226 modified "2023-10-14" @default.
• W4322758226 title "Tailoring the <i>p</i>‐Band Center of NS Pair for Accelerating High‐Performance Lithium–Oxygen Battery" @default.
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• W4322758226 doi "https://doi.org/10.1002/smll.202207461" @default.
• W4322758226 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36861365" @default.
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