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- W4322770942 endingPage "156" @default.
- W4322770942 startingPage "156" @default.
- W4322770942 abstract "Layered lithium transition metal (TM) oxides LiTMO2 (TM = Ni, Co, Mn, Al, etc.) are the most promising cathode materials for lithium-ion batteries because of their high energy density, good rate capability and moderate cost. However, the safety issue arising from the intrinsic thermal instability of nickel-based cathode materials is still a critical challenge for further applications in electric vehicles and energy storage power stations. The main reasons include side reactions between the highly reactive Ni3+/4+ and liquid electrolyte, oxygen release accompanied by structural phase transition, and internal microcrack propagation owing to the low strength of spherical secondary particles. Great efforts have been invested to modify nickel-based cathode materials such as stabilization of bulk structure by element doping, surface engineering, nanostructure design, and particle mono-crystallization. In this review, we summarize these advances and try to give an in-depth insight into the origin of the thermal instability of nickel-based cathode materials. More importantly, some effective strategies to improve thermal stability are outlined, expecting to accelerate the future development of layered TM oxides with high safety." @default.
- W4322770942 created "2023-03-03" @default.
- W4322770942 creator A5010738468 @default.
- W4322770942 creator A5022889656 @default.
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- W4322770942 creator A5043962546 @default.
- W4322770942 creator A5078065557 @default.
- W4322770942 creator A5082634019 @default.
- W4322770942 date "2023-03-01" @default.
- W4322770942 modified "2023-10-14" @default.
- W4322770942 title "Safety Issues of Layered Nickel-Based Cathode Materials for Lithium-Ion Batteries: Origin, Strategies and Prospects" @default.
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