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- W4323268182 abstract "Prussian blue analogues (PBAs), as the representative of Faradaic materials, has drawn extensive attention in capacitive deionization (CDI) for unique redox activity, open framework structure, and low-cost synthesis. However, the serious aggregation, low conductivity, and easy structural collapse of PBAs nanoparticles limit the practical application in CDI. Herein, the ternary composite Ni,[email protected]/PPy is flexibly constructed by integrating the collective advantages of Ni,Co-PBA, MXene, and PPy. In this configuration, MXene not only provides high conductivity but also acts as the good substrate for the in-situ homogeneous growth of Ni,Co-PBA nanoparticles. Furthermore, Ni,Co-PBA nanoparticles could effectively inhibit the self-stacking of MXene and facilitate fast ion intercalation. And the doping of Co in Ni,Co-PBA promotes the redox process by the pseudocapacitive contribution. Meanwhile, PPy contributes to accelerating ions transport rate and promoting the structural stability of MXene and Ni,Co-PBA. Consequently, the hybrid CDI cell AC//Ni,[email protected]/PPy delivers prominent desalination performance with the high salt adsorption capacity (38.7 mg g−1), rapid salt adsorption rate (10 mg g−1 min−1), low energy consumption (0.283 kWh kg−1-NaCl), and outstanding cyclic stability. Most importantly, the Ni,[email protected]/PPy electrode can reserve favorable structural integrity by the significant shielding effect of PPy to prevent Ni,Co-PBA from collapse and MXene from being oxidized." @default.
- W4323268182 created "2023-03-06" @default.
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- W4323268182 date "2023-06-01" @default.
- W4323268182 modified "2023-10-18" @default.
- W4323268182 title "Flexible structural construction of the ternary composite Ni,Co-Prussian blue analogue@MXene/polypyrrole for high-capacity capacitive deionization" @default.
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- W4323268182 doi "https://doi.org/10.1016/j.apsusc.2023.156926" @default.
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