Matches in SemOpenAlex for { <https://semopenalex.org/work/W4323308833> ?p ?o ?g. }
- W4323308833 endingPage "641" @default.
- W4323308833 startingPage "633" @default.
- W4323308833 abstract "Sluggish oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) kinetics inevitably impede the practical performance of rechargeable zinc–air batteries. Thus, combing the structural designability of transition metal-based electrocatalysts with anionic regulation is highly desired. Herein, mesoporous lamellar-stacked cobalt-based nanopiles with surface-sulfurization modification are elaborately designed and integrated with N/S co-doped graphene to build a robust OER/ORR bifunctional electrocatalyst. The lamellar-stacking mode of mesoporous nanosheets with abundant channels accelerates gas–liquid mass transfer, and partial-sulfurization of cobalt-based matrix surface efficiently improves the intrinsic OER activity. Meanwhile, N/S co-doped graphene further reinforces the ORR active sites while providing a stable conductive skeleton. As expected, this composite electrocatalyst delivers considerable bifunctional activity and stability, with an OER overpotential of 323 mV at 10 mA cm−2 and high durability. When applied in zinc–air batteries, remarkable ultralong-term stability over 4000 cycles and a maximum power density of 150.1 mW cm−2 are achieved. This work provides new insight into structure-composition synergistic design of rapid-kinetics OER/ORR bifunctional electrocatalyst for next-generation metal–air batteries." @default.
- W4323308833 created "2023-03-07" @default.
- W4323308833 creator A5002557721 @default.
- W4323308833 creator A5007471004 @default.
- W4323308833 creator A5018378779 @default.
- W4323308833 creator A5023784940 @default.
- W4323308833 creator A5066168744 @default.
- W4323308833 creator A5086515872 @default.
- W4323308833 creator A5086672489 @default.
- W4323308833 creator A5087259719 @default.
- W4323308833 creator A5087989101 @default.
- W4323308833 date "2023-06-01" @default.
- W4323308833 modified "2023-10-11" @default.
- W4323308833 title "Lamellar-stacked cobalt-based nanopiles integrated with nitrogen/sulfur co-doped graphene as a bifunctional electrocatalyst for ultralong-term zinc-air batteries" @default.
- W4323308833 cites W2157202716 @default.
- W4323308833 cites W2293908940 @default.
- W4323308833 cites W2395183679 @default.
- W4323308833 cites W2418436829 @default.
- W4323308833 cites W2506284908 @default.
- W4323308833 cites W2566737231 @default.
- W4323308833 cites W2567491100 @default.
- W4323308833 cites W2574394697 @default.
- W4323308833 cites W2614898114 @default.
- W4323308833 cites W2744576797 @default.
- W4323308833 cites W2755116647 @default.
- W4323308833 cites W2766269272 @default.
- W4323308833 cites W2791222711 @default.
- W4323308833 cites W2883284504 @default.
- W4323308833 cites W2905049004 @default.
- W4323308833 cites W2910927358 @default.
- W4323308833 cites W2923120862 @default.
- W4323308833 cites W2954060286 @default.
- W4323308833 cites W2959587863 @default.
- W4323308833 cites W2964006192 @default.
- W4323308833 cites W2965255951 @default.
- W4323308833 cites W2968536704 @default.
- W4323308833 cites W3004274313 @default.
- W4323308833 cites W3006196172 @default.
- W4323308833 cites W3015420320 @default.
- W4323308833 cites W3017351179 @default.
- W4323308833 cites W3021362005 @default.
- W4323308833 cites W3023836988 @default.
- W4323308833 cites W3045563046 @default.
- W4323308833 cites W3098110439 @default.
- W4323308833 cites W3127473628 @default.
- W4323308833 cites W3178528254 @default.
- W4323308833 cites W3178533589 @default.
- W4323308833 cites W3195891849 @default.
- W4323308833 cites W3209583458 @default.
- W4323308833 cites W4206965122 @default.
- W4323308833 cites W4220738009 @default.
- W4323308833 cites W4224060539 @default.
- W4323308833 cites W4280517210 @default.
- W4323308833 cites W4281635181 @default.
- W4323308833 cites W4281732829 @default.
- W4323308833 cites W4283123537 @default.
- W4323308833 cites W4284960284 @default.
- W4323308833 cites W4285412151 @default.
- W4323308833 cites W4307773098 @default.
- W4323308833 cites W4311021259 @default.
- W4323308833 cites W4313425505 @default.
- W4323308833 doi "https://doi.org/10.1016/j.jechem.2023.02.035" @default.
- W4323308833 hasPublicationYear "2023" @default.
- W4323308833 type Work @default.
- W4323308833 citedByCount "2" @default.
- W4323308833 countsByYear W43233088332023 @default.
- W4323308833 crossrefType "journal-article" @default.
- W4323308833 hasAuthorship W4323308833A5002557721 @default.
- W4323308833 hasAuthorship W4323308833A5007471004 @default.
- W4323308833 hasAuthorship W4323308833A5018378779 @default.
- W4323308833 hasAuthorship W4323308833A5023784940 @default.
- W4323308833 hasAuthorship W4323308833A5066168744 @default.
- W4323308833 hasAuthorship W4323308833A5086515872 @default.
- W4323308833 hasAuthorship W4323308833A5086672489 @default.
- W4323308833 hasAuthorship W4323308833A5087259719 @default.
- W4323308833 hasAuthorship W4323308833A5087989101 @default.
- W4323308833 hasConcept C127413603 @default.
- W4323308833 hasConcept C135473242 @default.
- W4323308833 hasConcept C147789679 @default.
- W4323308833 hasConcept C159985019 @default.
- W4323308833 hasConcept C161790260 @default.
- W4323308833 hasConcept C171250308 @default.
- W4323308833 hasConcept C17525397 @default.
- W4323308833 hasConcept C178790620 @default.
- W4323308833 hasConcept C179104552 @default.
- W4323308833 hasConcept C185592680 @default.
- W4323308833 hasConcept C186460083 @default.
- W4323308833 hasConcept C191897082 @default.
- W4323308833 hasConcept C192562407 @default.
- W4323308833 hasConcept C2780443040 @default.
- W4323308833 hasConcept C30080830 @default.
- W4323308833 hasConcept C33989665 @default.
- W4323308833 hasConcept C42360764 @default.
- W4323308833 hasConcept C515602321 @default.
- W4323308833 hasConcept C52859227 @default.
- W4323308833 hasConcept C77851909 @default.
- W4323308833 hasConcept C82776694 @default.
- W4323308833 hasConceptScore W4323308833C127413603 @default.