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- W4323310400 abstract "Solid electrolyte interphases (SEIs), which are formed by the decomposition of species in the inner Helmholtz plane (IHP) of the electrode surface, define the deposition behavior and cycling stability of Li metal anodes. Currently, the IHP is mainly tuned from electrolyte aspects. In this work, we report that the dominating species in the IHP could be readily controlled via surface dipoles. By self-assembling heteroatomic conjugated molecules on a Cu foil, we constructed a surface dipole that can increase the adsorption force of the Cu surface to anions, resulting in anion-rich IHP and an anion-derived SEI. The uniform nature of the self-assembled molecule layer and the robust anion-derived SEIs are conducive to uniform Li-deposited morphology, leading to a Li plating/stripping cycling Coulombic efficiency as high as 99.83%. This work sheds new light on tuning the electric double layer at the solid|liquid interface, which is of fundamental importance for the electrochemistry field." @default.
- W4323310400 created "2023-03-07" @default.
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- W4323310400 date "2023-03-01" @default.
- W4323310400 modified "2023-10-14" @default.
- W4323310400 title "Surface-dipole-directed formation of stable solid electrolyte interphase" @default.
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- W4323310400 doi "https://doi.org/10.1016/j.xcrp.2023.101324" @default.
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