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- W4323310919 abstract "We use general symmetry-based arguments to construct an effective model suitable for studying optical properties of lead-halide perovskites. To build the model, we identify an atomic-level interaction between electromagnetic fields and the spin degree of freedom that should be added to a minimally-coupled $mathbf{kcdot p}$ Hamiltonian. As a first application, we study two basic optical characteristics of the material: the Verdet constant and the refractive index. Beyond these linear characteristics of the material the model is suitable for calculating non-linear effects such as the third-order optical susceptibility. Analysis of this quantity shows that the geometrical properties of the spin-electric term imply isotropic optical response of the system, and that optical anisotropy of lead-halide perovskites is a manifestation of hopping of charge carriers. To illustrate this, we discuss third-harmonic generation." @default.
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- W4323310919 date "2023-03-06" @default.
- W4323310919 modified "2023-10-16" @default.
- W4323310919 title "Effective model for studying optical properties of lead halide perovskites" @default.
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- W4323310919 doi "https://doi.org/10.1103/physrevb.107.125201" @default.
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