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- W4323565581 abstract "Abstract We have synthesised and characterised 21 new ternary Pb(II) bromides with 16 different pyridine‐based organic cations by single crystal XRD measurements. The dominating composition is A PbBr 3 with 10 representatives, but also 6 examples for A Pb 2 Br 5 were found. The systematic variation of topological aspects of the organic cations allowed conclusions on the influence of N−H⋅⋅⋅Br hydrogen bridges on the connectivity and bonding situation of the Pb−Br polyhedra. Additionally, it turned out, that further weak ionic interactions can have an influence, if the formation of N−H⋅⋅⋅Br hydrogen bridges is hindered by steric effects. In general, the high versatility of the dominating PbBr 6 octahedra, and in some cases higher or lower coordination numbers, allows conclusions on the parameters that influence pattern and extent of the N−H⋅⋅⋅Br bridges as the strongest structure‐determining factor. Type and extent of N−H⋅⋅⋅Br bridges have also an impact on the distortion of the PbBr 6 octahedra ranging from nearly regular PbBr 6 octahedra to 2+2+2 and 1+2+2+1 patterns with significant lone pair activity. Finally, the connectivity mode of the octahedra relates to formation and strength of hydrogen bonds." @default.
- W4323565581 created "2023-03-09" @default.
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- W4323565581 date "2023-03-29" @default.
- W4323565581 modified "2023-10-18" @default.
- W4323565581 title "Interactions of Pyridine‐Based Organic Cations as Structure‐Determining Factors in Perovskite‐Related Compounds <i>A</i><sub>x</sub>Pb(II)<sub>y</sub>Br<sub>z</sub>" @default.
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- W4323565581 doi "https://doi.org/10.1002/ejic.202200671" @default.
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