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• W4323636741 abstract "Direct air capture (DAC) is important for achieving net-zero greenhouse gas emissions by 2050. However, the ultradilute atmospheric CO 2 concentration (~400 parts per million) poses a formidable hurdle for high CO 2 capture capacities using sorption-desorption processes. Here, we present a Lewis acid-base interaction–derived hybrid sorbent with polyamine-Cu(II) complex enabling over 5.0 mol of CO 2 capture/kg sorbent, nearly two to three times greater capacity than most of the DAC sorbents reported to date. The hybrid sorbent, such as other amine-based sorbents, is amenable to thermal desorption at less than 90°C. In addition, seawater was validated as a viable regenerant, and the desorbed CO 2 is simultaneously sequestered as innocuous, chemically stable alkalinity (NaHCO 3 ). The dual-mode regeneration offers unique flexibility and facilitates using oceans as decarbonizing sinks to widen DAC application opportunities." @default.
• W4323636741 created "2023-03-09" @default.
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• W4323636741 date "2023-03-10" @default.
• W4323636741 modified "2023-10-18" @default.
• W4323636741 title "Direct air capture (DAC) and sequestration of CO ₂ : Dramatic effect of coordinated Cu(II) onto a chelating weak base ion exchanger" @default.
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• W4323636741 doi "https://doi.org/10.1126/sciadv.adg1956" @default.
• W4323636741 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36888712" @default.
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