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• W4323645588 endingPage "9151" @default.
• W4323645588 startingPage "9140" @default.
• W4323645588 abstract "Asymmetric supercapacitors (ASCs) based on a battery-type anode and a capacitive-type cathode have been attracting extensive interest because of their high energy density. Herein, NiO nanosheets are hydrothermally deposited onto a V4C3TX substrate, which are then assembled into a 3D porous heterostructure hydrogel through a graphene oxide-assisted self-convergence hydrothermal process at low temperatures. The resultant hierarchical V4C3TX@NiO-RGO heterostructure hydrogel exhibits an ultrahigh specific capacitance of up to 1014.5 F g-1 at 1 A g-1. In addition, a defective reduced graphene oxide (DRGO) hydrogel is prepared using a cost-effective hydrothermal procedure followed by cobalt-catalyzed gasification, which shows a higher specific capacitance (258 F g-1 at 1 A g-1) than the untreated RGO hydrogel (176 F g-1). These two electrodes are then assembled into an ASC; the device features a stable operating voltage of 1.8 V, a maximum energy density of 86.22 W h kg-1 at 900 W kg-1, and excellent cycling stability at 96.4% capacitance retention after 10 000 cycles at 10 A g-1. The results from this work highlight the unique potential of MXene-based materials for the construction of high-performance ASCs." @default.
• W4323645588 created "2023-03-10" @default.
• W4323645588 creator A5002654282 @default.
• W4323645588 creator A5034717615 @default.
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• W4323645588 creator A5068316288 @default.
• W4323645588 creator A5074968253 @default.
• W4323645588 creator A5084696484 @default.
• W4323645588 date "2023-01-01" @default.
• W4323645588 modified "2023-10-04" @default.
• W4323645588 title "Hierarchical V₄C₃T_<i>X</i>@NiO-reduced graphene oxide heterostructure hydrogels and defective reduced graphene oxide hydrogels as free-standing anodes and cathodes for high-performance asymmetric supercapacitors" @default.
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• W4323645588 doi "https://doi.org/10.1039/d3cp00595j" @default.
• W4323645588 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36939188" @default.
• W4323645588 hasPublicationYear "2023" @default.
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