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- W4323651151 abstract "We explore the statistics of assembling soft-matter building blocks to investigate the uptake and encapsulation of cargo particles by carriers engulfing their load. While the such carrier-cargo complexes are important for many applications out of equilibrium, such as drug delivery and synthetic cell encapsulation, we uncover here the basic statistical physics in minimal hard-core-like models for particle uptake. Introducing an exactly solvable equilibrium model in one dimension, we demonstrate that the formation of carrier-cargo complexes can be largely tuned by both the cargo concentration and the carriers' interior size. These findings are intuitively explained by interpreting the internal free space (partition function) of the cargo inside a carrier as its engulfment strength, which can be mapped to an external control parameter (chemical potential) of an additional effective particle species. Such a mapping can be generally applied to account for attractive interactions, multiple cargo uptake and various carrier or cargo species. Within this effective equilibrium picture, we then suggest to employ effective non-Boltzmann occupation laws to describe the statistics of non-equilibrium particle uptake on the coarse-grained level. As a particular example, we put forward a Bose-Einstein-like phase transition associated with polydisperse carrier properties." @default.
- W4323651151 created "2023-03-10" @default.
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- W4323651151 date "2023-03-07" @default.
- W4323651151 modified "2023-10-17" @default.
- W4323651151 title "Statistics of carrier-cargo complexes" @default.
- W4323651151 doi "https://doi.org/10.48550/arxiv.2303.04005" @default.
- W4323651151 hasPublicationYear "2023" @default.
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