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• W4323664657 startingPage "154376" @default.
• W4323664657 abstract "Tritium population thermodynamics and transport kinetics critically define the tritium storage performance of zirconium tritides that can be used for a variety of nuclear applications including tritium-producing burnable absorber rods. Both thermodynamic and kinetic properties can be sensitive to grain sizes of materials and can be significantly altered by irradiated defects during operation under the reactor environments. A thorough experimental characterization of how these properties evolve under different reactor conditions and different initial grain structures is extremely challenging. Here molecular dynamics simulations are used to investigate tritium population and diffusion in zirconium with and without different planar symmetric and asymmetric tilt grain boundaries and irradiated defects. We found that in addition to trapping tritium, the most significant effect of planar grain boundaries is to increase tritium diffusivity on the boundary plane. Furthermore, fine grain structures are found to mitigate the change of tritium diffusivity due to irradiated point defects as these point defects are likely to migrate to and sink at grain boundaries." @default.
• W4323664657 created "2023-03-10" @default.
• W4323664657 creator A5026547934 @default.
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• W4323664657 date "2023-05-01" @default.
• W4323664657 modified "2023-09-30" @default.
• W4323664657 title "Molecular dynamics study of grain boundary and radiation effects on tritium population and diffusion in zirconium" @default.
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• W4323664657 doi "https://doi.org/10.1016/j.jnucmat.2023.154376" @default.
• W4323664657 hasPublicationYear "2023" @default.
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