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- W4323835903 abstract "In time-resolved pump-probe vibrational spectroscopy the internal stretch mode of polar molecules is utilized as a key observable to characterize the ultrafast dynamics of adsorbates on surfaces. The adsorbates non-adiabatic intermode couplings are the commonly accepted mechanisms behind the observed transient frequency shifts. Here, we study the CO/Pd(111) system with a robust theoretical framework that includes electron-hole pair excitations and electron-mediated coupling between the vibrational modes. A mechanism is revealed that screens the electron-phonon interaction and originates a blueshift under ultrafast non-equilibrium conditions. The results are explained in terms of the abrupt change in the density of states around the Fermi level, and are instrumental for understanding dynamics at multi-component surfaces involving localized and standard $s$ or $p$ states." @default.
- W4323835903 created "2023-03-11" @default.
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- W4323835903 date "2023-03-10" @default.
- W4323835903 modified "2023-09-25" @default.
- W4323835903 title "Anomalous transient blueshift in the internal stretch mode of CO/Pd(111)" @default.
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- W4323835903 doi "https://doi.org/10.1103/physrevb.107.l121404" @default.
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