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• W4324018097 abstract "One-directional electron transport between a photocatalyst and redox mediator is crucial for achieving highly active Z-scheme water-splitting photocatalysis. Herein, a photoredox cascade catalyst that artificially mimics the electron transport chain in natural photosynthesis was synthesized from a Pt-TiO2 nanoparticle catalyst, two photosensitizers (RuCP6 and RuP6), and a visible-light-transparent electron mediator (HCRu). During photocatalytic hydrogen evolution in the presence of a redox-reversible electron donor, [Co(bpy)3]2+ (bpy = 2,2'-bipyridine), the HCRu-Zr-RuCP6-Zr-RuP6@Pt-TiO2 (PRCC-1) photocatalyst exhibited the highest reported initial (1 h) apparent quantum yield (iAQY = 2.23%) of dye-sensitized TiO2 photocatalysts to date. Furthermore, PRCC-1 successfully produced hydrogen when using hydroquinone monosulfonate (H2QS-) as the hydrogen source." @default.
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• W4324018097 date "2023-03-13" @default.
• W4324018097 modified "2023-10-05" @default.
• W4324018097 title "Efficient Hydrogen Production by a Photoredox Cascade Catalyst Comprising Dual Photosensitizers and a Transparent Electron Mediator" @default.
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• W4324018097 doi "https://doi.org/10.1021/jacs.2c13687" @default.
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