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- W4324139211 abstract "n-Type conjugated polymers (CPs) are crucial in the applications of organic electronics. Direct coupling of electron-deficient C−H monomer via selective C−H activation, namely C−H/C−H oxidative direct arylation polycondensation (Oxi-DArP), is an ideal approach toward such CPs. Herein, Oxi-DArP is firstly adopted to synthesize a high-performance n-type CP using a newly developed monomer, i.e., 3,6-di(thiazol-5-yl)-diketopyrrolopyrrole (Tz-5-DPP). Tz-5-DPP based homopolymer PTz-5-DPP with a molecular weight of 22 kDa has been synthesized via Oxi-DArP. After n-doping, PTz-5-DPP films exhibited electric conductivity values up to 8 S cm−1 and power factors (PFs) up to 106 μW m−1 K−2. Notably, this PF value is the highest for n-type polymer thermoelectric materials to date. The Oxi-DArP synthesis and the excellent n-type performance of the polymer make this work an important step toward the straightforward and sustainable preparation of high-performance n-type polymer semiconductors." @default.
- W4324139211 created "2023-03-15" @default.
- W4324139211 creator A5011728561 @default.
- W4324139211 creator A5014243683 @default.
- W4324139211 creator A5021773001 @default.
- W4324139211 creator A5060510290 @default.
- W4324139211 creator A5084903568 @default.
- W4324139211 creator A5085902993 @default.
- W4324139211 date "2023-04-07" @default.
- W4324139211 modified "2023-10-13" @default.
- W4324139211 title "A High‐Performance n‐Type Thermoelectric Polymer from C−H/C−H Oxidative Direct Arylation Polycondensation" @default.
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