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- W4324143048 abstract "Abstract Hydrogen is a promising alternative to fossil fuels that can reduce greenhouse gas emissions. Decoupled water electrolysis system using a reversible proton storage redox mediator, where the oxygen evolution reaction and hydrogen evolution reaction are separated in time and space, is an effective approach to producing hydrogen gas with high purity, high flexibility, and low cost. To realize fast hydrogen production in such a system, a redox mediator capable of releasing protons rapidly is required. Herein, α‐MoO 3 , with an ultrafast proton transfer property that can be explained by a dense hydrogen bond network in the lattice oxygen arrays of HxMoO 3 , is examined as a high‐rate redox mediator for fast hydrogen production in acidic electrolytes. The α‐MoO 3 redox mediator shows both a large capacity of 204 mAh g −1 and fast hydrogen production at a current rate of 10 A cm −2 (≈153 A g −1 ), outperforming most of the previously reported solid‐state redox mediators." @default.
- W4324143048 created "2023-03-15" @default.
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- W4324143048 date "2023-03-14" @default.
- W4324143048 modified "2023-09-30" @default.
- W4324143048 title "High‐rate Decoupled Water Electrolysis System Integrated with α‐MoO<sub>3</sub> as a Redox Mediator with Fast Anhydrous Proton Kinetics" @default.
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- W4324143048 doi "https://doi.org/10.1002/adfm.202214466" @default.
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