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- W4324348646 abstract "Metal-organic frameworks (MOFs) with functional groups are developed for the nanoconfinement of chlorine by chemisorption in a rechargeable Li-Cl2 battery. Predicted by theoretical calculations, highly porous MOF functionalized with –NH2 groups, namely UiO-66-NH2, is screened out as a model to apply in the Li-Cl2 battery. The Li-Cl2 battery using NH2-functionalized MOF (Li-Cl2@MOF) demonstrates high specific capacities of up to 2,000 mAh/g and is highly stable for 500 cycles under a specific capacity of 1,000 mAh/g at room temperature. It also exhibits superior low-temperature performance, displaying a high voltage of 3.5 V and a Coulombic efficiency (CE) of 99.7% with 300 stable cycles under a capacity of 1,000 mAh/g at −25°C. Furthermore, the Li-Cl2@MOF cell exhibits a high areal capacity of 4.4 mAh/cm2 in coin cells and a CE of 99% for over 120 cycles in large-scale pouch cells. This work provides opportunities for the promising application of functionalized MOFs as cathodes in rechargeable Li-Cl2 batteries." @default.
- W4324348646 created "2023-03-16" @default.
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- W4324348646 date "2023-03-01" @default.
- W4324348646 modified "2023-10-17" @default.
- W4324348646 title "Metal-organic frameworks for nanoconfinement of chlorine in rechargeable lithium-chlorine batteries" @default.
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- W4324348646 doi "https://doi.org/10.1016/j.joule.2023.02.010" @default.
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