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- W4324363441 abstract "The mechanism of the recently reported catalyzed asymmetric hydrogenation of enyne 1 catalyzed by the Co-(R,R)-QuinoxP* complex was studied by DFT. Conceivable pathways for the Co(I)-Co(III) mechanism were computed together with a Co(0)-Co(II) catalytic cycle. It is commonly assumed that the exact nature of the chemical transformations taking place along the actually operating catalytic pathway determine the sense and level of enantioselection of the catalytic reaction. In this work, two chemically different mechanisms reproduced the experimentally observed perfect stereoselection of the same handedness. Moreover, the relative stabilities of the transition states of the stereo induction stages were controlled via exactly the same weak disperse interactions between the catalyst and the substrate." @default.
- W4324363441 created "2023-03-16" @default.
- W4324363441 creator A5081669336 @default.
- W4324363441 date "2023-03-14" @default.
- W4324363441 modified "2023-09-26" @default.
- W4324363441 title "Co-Catalyzed Asymmetric Hydrogenation. The Same Enantioselection Pattern for Different Mechanisms" @default.
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- W4324363441 doi "https://doi.org/10.3390/ijms24065568" @default.
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- W4324363441 hasPublicationYear "2023" @default.
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